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Journal Articles

An Analytical model to decompose mass transfer and chemical process contributions to molecular iodine release from aqueous phase under severe accident conditions

Zablackaite, G.; Shiotsu, Hiroyuki; Kido, Kentaro; Sugiyama, Tomoyuki

Nuclear Engineering and Technology, 56(2), p.536 - 545, 2024/02

 Times Cited Count:0 Percentile:0.08(Nuclear Science & Technology)

Journal Articles

Effect of fuel particle size on consequences of criticality accidents in water-moderated solid fuel particle dispersion system

Fukuda, Kodai; Yamane, Yuichi

Journal of Nuclear Science and Technology, 60(12), p.1514 - 1525, 2023/12

 Times Cited Count:1 Percentile:68.31(Nuclear Science & Technology)

This study aims to clarify the effect of fuel particle radius on the criticality transient behavior and the total number of fissions in water-moderated solid fuel dispersion systems. Neutronics/thermal hydraulics-coupled kinetics analysis was performed in a hypothetical fuel debris system, where small fuel particles aggregate in water and become supercritical. Results showed that the number of fissions is 10 times larger when the fuel particle radius is reduced by one order of magnitude under conditions where heat transfer, i.e. from fuel to water, is emphasized. Moreover, there is a possibility that lower reactivity could give a larger number of fissions when the fuel particle size is very small. In addition, the number of fissions may be overestimated or underestimated to an unexpected extent unless appropriate fuel particle size is set on the analysis.

Journal Articles

Double diffusive dissolution model of UO$$_{2}$$ pellet in molten Zr cladding

Ito, Ayumi*; Yamashita, Susumu; Tasaki, Yudai; Kakiuchi, Kazuo; Kobayashi, Yoshinao*

Journal of Nuclear Science and Technology, 60(4), p.450 - 459, 2023/04

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

Journal Articles

Unusually kinetically inert monocationic neptunyl complex with a fluorescein-modified 1,10-phenanthroline-2,9-dicarboxylate ligand; Specific separation and detection in gel electrophoresis

Yamagata, Kazuhito*; Ouchi, Kazuki; Marumo, Kazuki*; Tasaki-Handa, Yuiko*; Haraga, Tomoko; Saito, Shingo*

Inorganic Chemistry, 62(2), p.730 - 738, 2023/01

 Times Cited Count:3 Percentile:74.01(Chemistry, Inorganic & Nuclear)

The inert NpO$$_{2}$$$$^{+}$$ complex with a fluorescein-modified phenanthroline-2,9-dicarboxylic acid was found by kinetic selection using polyacrylamide gel electrophoresis (PAGE) from a small chemical library. The small spontaneous dissociation rate constant of 8$$times$$10$$^{-6}$$ s$$^{-1}$$ (the half-life of 23 hours) was determined. This is the singly-charged NpO$$_{2}$$$$^{+}$$ complex exhibiting unusual kinetic inertness in aqueous solution, one million times slower than widely accepted fast kinetics of neptunyl complexes. Selective fluorescence detection of NpO$$_{2}$$$$^{+}$$ was achieved in PAGE with a detection limit of 68 pmol dm$$^{-3}$$(17 fg). This system was successfully applied to simulated spent nuclear fuel and high-level radioactive waste samples.

Journal Articles

Reactivity estimation based on the linear equation of characteristic time profile of power in subcritical quasi-steady state

Yamane, Yuichi

Journal of Nuclear Science and Technology, 59(11), p.1331 - 1344, 2022/11

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

The reactivity was estimated from a time profile of neutron count rate or a simulated data in a quasi-steady state after sudden change of reactivity or external neutron source strength. The estimation was based on the equation of power in subcritical quasi-steady state. The purpose of the study is to develop the method of timely reactivity estimation from complicated time profile of neutron count rate. The developed method was applied to the data simulating neutron count rate created by using one-point kinetics code, AGNES, and Poisson-distributed random noise and to the transient subcritical experiment data measured by using TRACY. The result shows that the difference of the estimated and reference value was within about 5% or less for ($$rho$$${$}$ $$>$$ -1) for simulated data and within about 7% or less for $$rho$$${$}$ $$simeq$$ -1.4 and -3.1 for the experimental data. It was also shown that the possibility of the reactivity estimation several ten seconds after the status change.

Journal Articles

Star-polymer-DNA gels showing highly predictable and tunable mechanical responses

Ohira, Masashi*; Katashima, Takuya*; Naito, Mitsuru*; Aoki, Daisuke*; Yoshikawa, Yusuke*; Iwase, Hiroki*; Takata, Shinichi; Miyata, Kanjiro*; Chung, U.-I.*; Sakai, Takamasa*; et al.

Advanced Materials, 34(13), p.2108818_1 - 2108818_9, 2022/01

 Times Cited Count:13 Percentile:89.15(Chemistry, Multidisciplinary)

Journal Articles

Calculation of transient parameters of the integral kinetic model with delayed neutrons for space-dependent kinetic analysis of coupled reactors

Takezawa, Hiroki*; Tuya, D.; Obara, Toru*

Nuclear Science and Engineering, 195(11), p.1236 - 1246, 2021/11

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

This study introduces new methodologies for integrating fission reactions induced by delayed neutrons into the Multi-Region Integral Kinetic (MIK) code by using a Monte Carlo neutron transport calculation. First, it was confirmed that it is feasible to solve the Integral Kinetic Model (IKM) with delayed neutrons by the forward Euler discretization method in terms of the number of time steps. This can be done with the help of the law of radioactive decay to reflect the delay in the emission of delayed neutrons in the discretized IKM. Second, a new Monte Carlo-based methodology was introduced for calculating the cumulative distribution functions of secondary fission induced by prompt and delayed neutrons. These functions are necessary for the discretized IKM. The results of preliminary verification using the Godiva reactor confirmed the applicability of the new Monte Carlo-based methodology.

Journal Articles

Isotope and plasma size scaling in ion temperature gradient driven turbulence

Idomura, Yasuhiro

Europhysics Conference Abstracts (Internet), 45A, 4 Pages, 2021/06

This work presents the impacts of the hydrogen isotope mass and the normalized plasma size on confinement of hydrogen (H) and deuterium (D) plasmas dominated by ion temperature gradient driven turbulence. Numerical experiments of H and D plasmas with ion and electron heating conditions were conducted using the Gyrokinetic Toroidal 5D full- f Eulerian code GT5D. The energy confinement time in the ion heated numerical experiments was almost independent of isotope mass, and the energy confinement was determined mainly by the normalized plasma size or the plasma size divided by the ion gyro radius, indicating an impact of non-local transport. On the other hand, the electron heated numerical experiments showed a clear isotope mass dependency. In addition to the plasma size effect, the isotope mass dependency of the collisional energy transfer from electrons to ions changes the ion heat flux and the turbulence intensity, leading to the degradation of confinement in H plasmas. These results qualitatively agree with the hydrogen isotope scaling in experiments.

Journal Articles

Acceleration of fusion plasma turbulence simulations using the mixed-precision communication-avoiding Krylov method

Idomura, Yasuhiro; Ina, Takuya*; Ali, Y.*; Imamura, Toshiyuki*

Proceedings of International Conference for High Performance Computing, Networking, Storage, and Analysis (SC 2020) (Internet), p.1318 - 1330, 2020/11

 Times Cited Count:1 Percentile:36.4(Computer Science, Information Systems)

The multi-scale full-$$f$$ simulation of the next generation experimental fusion reactor ITER based on a five dimensional (5D) gyrokinetic model is one of the most computationally demanding problems in fusion science. In this work, a Gyrokinetic Toroidal 5D Eulerian code (GT5D) is accelerated by a new mixed-precision communication-avoiding (CA) Krylov method. The bottleneck of global collective communication on accelerated computing platforms is resolved using a CA Krylov method. In addition, a new FP16 preconditioner, which is designed using the new support for FP16 SIMD operations on A64FX, reduces both the number of iterations (halo data communication) and the computational cost. The performance of the proposed method for ITER size simulations with 0.1 trillion grids on 1,440 CPUs/GPUs on Fugaku and Summit shows 2.8x and 1.9x speedups respectively from the conventional non-CA Krylov method, and excellent strong scaling is obtained up to 5,760 CPUs/GPUs.

Journal Articles

A Linear Equation of characteristic time profile of power in subcritical quasi-steady state

Yamane, Yuichi

Journal of Nuclear Science and Technology, 57(8), p.926 - 931, 2020/08

 Times Cited Count:1 Percentile:11.8(Nuclear Science & Technology)

An equation of power in subcritical quasi-steady state has been derived based on one-point kinetics equations for the purpose of utilizing it for the development of timely reactivity estimation from complicated time profile of neutron count rate. It linearly relates power, $$P$$, to a new variable $$q$$, which is a function of time differential of the power. It has been confirmed by using one-point kinetics code, AGNES, that the calculated points ($$q, P$$) are perfectly in a line described by the new equation and that points ($$q, P$$) calculated from transient subcritical experiments by using TRACY made a line with a slope indicated by the new equation.

Journal Articles

Behavior of high-burnup advanced LWR fuel cladding tubes under LOCA conditions

Narukawa, Takafumi; Amaya, Masaki

Proceedings of International Nuclear Fuel Cycle Conference / Light Water Reactor Fuel Performance Conference (Global/Top Fuel 2019) (USB Flash Drive), p.912 - 921, 2019/09

Journal Articles

Oxidation behavior of high-burnup advanced fuel cladding tubes in high-temperature steam

Narukawa, Takafumi; Amaya, Masaki

Journal of Nuclear Science and Technology, 56(7), p.650 - 660, 2019/07

 Times Cited Count:11 Percentile:76.81(Nuclear Science & Technology)

Journal Articles

Synergy of turbulent and neoclassical transport through poloidal convective cells

Asahi, Yuichi*; Grandgirard, V.*; Sarazin, Y.*; Donnel, P.*; Garbet, X.*; Idomura, Yasuhiro; Dif-Pradalier, G.*; Latu, G.*

Plasma Physics and Controlled Fusion, 61(6), p.065015_1 - 065015_15, 2019/05

 Times Cited Count:4 Percentile:26.6(Physics, Fluids & Plasmas)

The role of poloidal convective cells on transport processes is studied with the full-F gyrokinetic code GYSELA. For this purpose, we apply a numerical filter to convective cells and compare the simulation results with and without the filter. The energy flux driven by the magnetic drifts turns out to be reduced by a factor of about 2 once the numerical filter is applied. A careful analysis reveals that the frequency spectrum of the convective cells is well-correlated with that of the turbulent Reynolds stress tensor, giving credit to their turbulence-driven origin. The impact of convective cells can be interpreted as a synergy between turbulence and neoclassical dynamics.

Journal Articles

Thorium oxide dissolution in HNO$$_{3}$$-HF mixture; Kinetics and mechanism

Simonnet, M.; Barr$'e$, N.*; Drot, R.*; Le Naour, C.*; Sladkov, V.*; Delpech, S.*

Radiochimica Acta, 107(4), p.289 - 297, 2019/04

 Times Cited Count:3 Percentile:21.22(Chemistry, Inorganic & Nuclear)

Journal Articles

The Influence of the air fraction in steam on the growth of the columnar oxide and the adjacent $$alpha$$-Zr(O) layer on Zry-4 fuel cladding at 1273 and 1473 K

Negyesi, M.; Amaya, Masaki

Annals of Nuclear Energy, 114, p.52 - 65, 2018/04

 Times Cited Count:6 Percentile:52.24(Nuclear Science & Technology)

Journal Articles

Evaluation of feedback reactivity coefficients by inverse kinetics in Monju

Kitano, Akihiro; Nakajima, Ken*

Proceedings of 2018 International Congress on Advances in Nuclear Power Plants (ICAPP 2018) (CD-ROM), p.1205 - 1210, 2018/04

The feedback reactivity is taken into account in fast reactor core design especially in order to make the power coefficient negative, which is required to be confirmed in the operation. In the feedback reactivity experiment, the positive reactivity was inserted in the critical state at zero power, and the thermal data, such as reactor power and the R/V inlet temperature, was acquired until the power got stable by the feedback reactivity. In the conventional study, only two critical points in an experiment are available for evaluation of the feedback reactivity coefficients. This method needs three days for evaluation. The advanced method based on the inverse kinetics is newly applied in this work using the more extensive data. It is confirmed that this approach can evaluate the feedback reactivity coefficients in one experiment.

Journal Articles

Oxidation kinetics of Zry-4 fuel cladding in mixed steam-air atmospheres at temperatures of 1273 - 1473 K

Negyesi, M.; Amaya, Masaki

Journal of Nuclear Science and Technology, 54(10), p.1143 - 1155, 2017/10

 Times Cited Count:6 Percentile:50.9(Nuclear Science & Technology)

Journal Articles

Development of experimental and analytical technologies for fission product chemistry under LWR severe accident condition

Miyahara, Naoya; Miwa, Shuhei; Nakajima, Kunihisa; Osaka, Masahiko

Proceedings of 2017 Water Reactor Fuel Performance Meeting (WRFPM 2017) (USB Flash Drive), 9 Pages, 2017/09

This paper presents the development of a reproductive experimental setup for FP release and transport and an analysis tool considering chemical reaction kinetics for the construction of the FP chemistry database. The performance test of the reproductive experimental setup TeRRa using CsI compounds show that TeRRa can reproduce well a FP chemistry-related behavior such as aerosol formation, growth and deposition behavior. An analytical tool has been developed based on the commercial ANSYS-FLUENT code. Some additional models was added to evaluate detailed FP chemistry during release and transport in this study. A test analysis simulating the CsI heating test in steam atmosphere was carried out to demonstrate the performance of the improved code. The result shows the appropriateness of the additional models.

Journal Articles

Determination of reactivity and neutron flux using modified neural network for HTGR

Subekti, M.*; Kudo, Kazuhiko*; Nabeshima, Kunihiko; Takamatsu, Kuniyoshi

Atom Indonesia, 43(2), p.93 - 102, 2017/08

Reactor kinetics based on point kinetic model have been generally applied as the standard method for neutronics codes. As the central control rod (C-CR) withdrawal test has demonstrated in a prismatic core of HTTR, the transient calculation of kinetic parameter, such as reactivity and neutron fluxes, requires a new method to shorten calculation-process time. Development of neural network method was applied to point kinetic model as the necessity of real-time calculation that could work in parallel with the digital reactivity meter. The combination of TDNN and Jordan RNN, such as TD-Jordan RNN, was the result of the modeling approach. The application of TD-Jordan RNN with adequate learning, tested offline, determined results accurately even when signal inputs were noisy. Furthermore, the preprocessing for neural network input utilized noise reduction as one of the equations to transform two of twelve time-delayed inputs into power corrected inputs.

Journal Articles

Optimization of fusion kernels on accelerators with indirect or strided memory access patterns

Asahi, Yuichi*; Latu, G.*; Ina, Takuya; Idomura, Yasuhiro; Grandgirard, V.*; Garbet, X.*

IEEE Transactions on Parallel and Distributed Systems, 28(7), p.1974 - 1988, 2017/07

 Times Cited Count:7 Percentile:55.15(Computer Science, Theory & Methods)

High-dimensional stencil computation from fusion plasma turbulence codes involving complex memory access patterns, the indirect memory access in a Semi-Lagrangian scheme and the strided memory access in a Finite-Difference scheme, are optimized on accelerators such as GPGPUs and Xeon Phi coprocessors. On both devices, the Array of Structure of Array (AoSoA) data layout is preferable for contiguous memory accesses. It is shown that the effective local cache usage by improving spatial and temporal data locality is critical on Xeon Phi. On GPGPU, the texture memory usage improves the performance of the indirect memory accesses in the Semi-Lagrangian scheme. Thanks to these optimizations, the fusion kernels on accelerators become 1.4x - 8.1x faster than those on Sandy Bridge (CPU).

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